Storming Media: Pentagon Reports and DocumentsPentagon Reports: Fast. Definitive. Complete.     
New Account »
Forgot Password?
Advanced Search »
ChemistryPhysical Chemistry

Matrix Isolation Spectroscopy Applied to Positron Moderatioin in Cryogenic Solids

Authors: Mario E. Fajardo; Christopher D. Molek; C. M. Lindsay; AIR FORCE RESEARCH LAB EGLIN AFB FL MUNITIONS DIRECTORATE
Abstract:
We report results of Matrix Isolation Spectroscopy (MIS) experiments performed on working cryogenic rare gas solid (RGS) positron (e+) moderators. The e+ is the antiparticle to the electron,1-3 and positrons are produced by energetic processes that result in very broad kinetic energy distributions (KEDs) - typically spanning hundreds of thousands of electron volts (eV). Trapping and manipulating e+ with electromagnetic fields requires narrowing these KEDs below a few eV, which is accomplished via velocity-dependent interactions in a normal matter "moderator". A fast e+ entering a wide bandgap dielectric RGS moderator slows rapidly within the first ~ picosecond, producing a track of ionized and electronically excited species. However, once KEe+ drops below the ~ 10 eV minimum required for generating such excitations, these interactions abruptly switch off, and the e+ enters a phase of "hyperthermal diffusion" that can last for nanoseconds. Positrons that reach a free surface of the moderator before annihilating with an electron may escape into vacuum where they can be manipulated. The best known e+ moderator is cryogenic solid Ne, which still only delivers efficiencies < 1 %; the other 99+ % of the nascent fast e+ are wasted. Additionally, the RGS moderator efficiency is known to decrease during operation, which is attributed variously to the buildup of radiation damage, and/or to contamination of the moderator surface by residual gas deposition. We constructed a novel apparatus that permits optical access to a working cryogenic solid moderator. Our original motivation was to test our hypothesis that solid parahydrogen (pH2) should be an even better e+ moderator than solid Ne, while simultaneously monitoring the condition of the moderators by infrared (IR) absorption spectroscopy. Unfortunately, the performance of our ortho/para hydrogen converter (o/p convert

Limitations: APPROVED FOR PUBLIC RELEASE
Description: Briefing charts
Pages: 40
Report Date: JUL 2011
Contract Number: AFRL-RW-EG-TP-2011-024
Report Number: A245745
Keywords relating to this report:
ABSORPTION SPECTRA
ACCESS
BROADBAND
CONTAMINATION
CRYOGENICS
DEPOSITION
DIFFUSION
ELECTROMAGNETIC FIELDS
ENERGETIC PROPERTIES
ENERGY GAPS
GASES
HIGH TEMPERATURE
MATRIX THEORY
OPTICAL PROPERTIES
POSITRONS
RADIATION DAMAGE
RARE GASES
REPORTS
RESIDUALS
SOLIDIFIED GASES
SPECTROSCOPY
VOLTAGE
Email This Abstract